发表状态 | 已发表Published |
题名 | Simultaneous removal of triadimefon and dinotefuran by a new biochar-based magnesium oxide composite in water: Performances and mechanism |
作者 | |
发表日期 | 2024-05-25 |
发表期刊 | Separation and Purification Technology
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ISSN/eISSN | 1383-5866 |
卷号 | 336 |
摘要 | In recent years, the ecological security has been seriously threatened by the residues of pesticides in the environment. In this study, a new biochar-based magnesium oxide composite (MTBC) was successfully prepared using Traditional Chinese Medicine residues and MgCl solution, and then applied for the removal of triadimefon (TDF) and/or dinotefuran (DIN) in water. Batch experiments results indicated that 86.42 and 87.86 % of TDF and DIN removals could be obtained by MTBC within 120 min, respectively. The TDF adsorption process was proved to be well fitted with the pseudo-second-order kinetic, Elovich, liquid film diffusion, Intra-particle diffusion and Langmuir isothermal models. The TDF adsorption by MTBC was a spontaneous endothermic reaction, and chemical adsorption process was dominant. The inhibitory of the coexisting anions on TDF removal followed the order of SO<Cl<HPO<HCO. Both TDF and DIN could be simultaneously removed by MTBC at the certain concentrations levels. The possible removal mechanism for the adsorption of TDF and DIN by MTBC was proposed, both TDF and DIN were rapidly distributed and adsorbed on MTBC surface, then diffused into the interior pores structure and were finally adsorbed on MTBC through various reaction processes. The TDF removal process might be involved with hydrogen bonding, π-π interaction, pore filling and electrostatic interaction, while DIN removal might be involved with hydrogen bonding, pore filling and electrostatic interaction. These findings suggested that biochar-based magnesium oxide composite was an effective adsorbent for the remediation of agricultural effluents containing TDF and DIN. |
关键词 | Adsorption Biochar Dinotefuran Pesticides Simultaneous removal Triadimefon |
DOI | 10.1016/j.seppur.2023.126213 |
URL | 查看来源 |
收录类别 | SCIE |
语种 | 英语English |
WOS研究方向 | Engineering |
WOS类目 | Engineering, Chemical |
WOS记录号 | WOS:001155842600001 |
Scopus入藏号 | 2-s2.0-85181824945 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | https://repository.uic.edu.cn/handle/39GCC9TT/11447 |
专题 | 北师香港浸会大学 |
通讯作者 | Guo, Peng Ran; Diao, Zeng Hui |
作者单位 | 1.Guangdong Provincial Key Laboratory of Chemical Measurement and Emergency Test Technology,Institute of Analysis,Guangdong Academy of Sciences,Guangzhou,510070,China 2.Zhongkai University of Agriculture and Engineering,Guangzhou,510225,China 3.Beijing Normal University-Hong Kong Baptist University United International College,Zhuhai,519087,China 4.Guangzhou University,Guangzhou,510006,China |
推荐引用方式 GB/T 7714 | Chen, Xie,Yao, Xiao Wen,Diao, Yiet al. Simultaneous removal of triadimefon and dinotefuran by a new biochar-based magnesium oxide composite in water: Performances and mechanism[J]. Separation and Purification Technology, 2024, 336. |
APA | Chen, Xie., Yao, Xiao Wen., Diao, Yi., Liu, Hui., Chen, Man Li., .. & Diao, Zeng Hui. (2024). Simultaneous removal of triadimefon and dinotefuran by a new biochar-based magnesium oxide composite in water: Performances and mechanism. Separation and Purification Technology, 336. |
MLA | Chen, Xie,et al."Simultaneous removal of triadimefon and dinotefuran by a new biochar-based magnesium oxide composite in water: Performances and mechanism". Separation and Purification Technology 336(2024). |
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