Status | 已发表Published |
Title | Antibiofouling polyethersulfone ultrafiltration membranes functionalized with MoS2 nanosheets and self-cleaning with hydrogen peroxide |
Creator | |
Date Issued | 2023-12-01 |
Source Publication | Journal of Environmental Chemical Engineering
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Volume | 11Issue:6 |
Abstract | The development of biofouling mitigation and cleaning strategy is of paramount importance for ultrafiltration (UF) membrane biofouling. In this study, polyethersulfone (PES) UF membrane was functionalized, namely MoS/PES composite membrane. The MoS/PES composite membrane exhibited superior antifouling property as evidenced by antibacterial circle, static and dynamic biofouling experiments. The permeate fluxes of the pristine PES and MoS/PES composite membrane respectively decreased by 76% and 31% at the end of 3-h filtration. After exposure of E. coli to MoS, inhibited cell growth led to reduced membrane biofouling. The biofilm formation was retarded under the dynamic flow condition, which were further confirmed by Scanning Electron Microscopy (SEM) and Confocal Laser Scanning Microscopy (CLSM) observations. As for the enhanced biofouling removal by cleaning with HO, 62% of the flux recovery rate for the MoS/PES composite membrane was much higher than the pristine PES membrane (24%). The peroxidase-like properties of MoS were responsible for the enhancement of the superior cleaning performance. The use of HO to trigger the in-situ catalytic function of the MoS nano-enzyme generated more ROS and O for inducing bacterial cells death and facilitating detachment of biofilm. This work will be helpful to provide important insights into developing more effective strategies for biofouling control and cleaning using advanced nanomaterials in membrane-based water treatment processes. |
Keyword | Antibacterial activity Biofouling Membrane cleaning MoS2 nanosheets |
DOI | 10.1016/j.jece.2023.111571 |
URL | View source |
Indexed By | SCIE |
Language | 英语English |
WOS Research Area | Engineering |
WOS Subject | Engineering, Environmental ; Engineering, Chemical |
WOS ID | WOS:001139405800001 |
Scopus ID | 2-s2.0-85178097207 |
Citation statistics | |
Document Type | Journal article |
Identifier | http://repository.uic.edu.cn/handle/39GCC9TT/11083 |
Collection | Beijing Normal-Hong Kong Baptist University |
Corresponding Author | Liu, Yang |
Affiliation | 1.Joint Research Centre for Protective Infrastructure Technology and Environmental Green Bioprocess,School of Environmental and Municipal Engineering,Tianjin Chengjian University,Tianjin,NO.26, Jinjing Rd, Xiqing District,300384,China 2.Tianjin Key Laboratory of Aquatic Science and Technology,School of Environmental and Municipal Engineering,Tianjin Chengjian University,Tianjin,NO.26, Jinjing Rd, Xiqing District,300384,China 3.Environmental Science Program,Department of Life Sciences,Beijing Normal University-Hong Kong Baptist University United International College,Zhuhai,No. 2000 Jintong Road, Tangjiawan,519087,China 4.Engineering Laboratory of Low-Carbon Unconventional Water Resources Utilization and Water Quality Assurance,College of Environmental Science and Engineering,Nankai University,Tianjin,300350,China |
Recommended Citation GB/T 7714 | Huang, Xuanlin,Liu, Yang,Zhao, Yingcanet al. Antibiofouling polyethersulfone ultrafiltration membranes functionalized with MoS2 nanosheets and self-cleaning with hydrogen peroxide[J]. Journal of Environmental Chemical Engineering, 2023, 11(6). |
APA | Huang, Xuanlin, Liu, Yang, Zhao, Yingcan, Zhang, Xinbo, & Zhang, Xiaoyuan. (2023). Antibiofouling polyethersulfone ultrafiltration membranes functionalized with MoS2 nanosheets and self-cleaning with hydrogen peroxide. Journal of Environmental Chemical Engineering, 11(6). |
MLA | Huang, Xuanlin,et al."Antibiofouling polyethersulfone ultrafiltration membranes functionalized with MoS2 nanosheets and self-cleaning with hydrogen peroxide". Journal of Environmental Chemical Engineering 11.6(2023). |
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