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Status已发表Published
TitleAntibiofouling polyethersulfone ultrafiltration membranes functionalized with MoS2 nanosheets and self-cleaning with hydrogen peroxide
Creator
Date Issued2023-12-01
Source PublicationJournal of Environmental Chemical Engineering
Volume11Issue:6
Abstract

The development of biofouling mitigation and cleaning strategy is of paramount importance for ultrafiltration (UF) membrane biofouling. In this study, polyethersulfone (PES) UF membrane was functionalized, namely MoS/PES composite membrane. The MoS/PES composite membrane exhibited superior antifouling property as evidenced by antibacterial circle, static and dynamic biofouling experiments. The permeate fluxes of the pristine PES and MoS/PES composite membrane respectively decreased by 76% and 31% at the end of 3-h filtration. After exposure of E. coli to MoS, inhibited cell growth led to reduced membrane biofouling. The biofilm formation was retarded under the dynamic flow condition, which were further confirmed by Scanning Electron Microscopy (SEM) and Confocal Laser Scanning Microscopy (CLSM) observations. As for the enhanced biofouling removal by cleaning with HO, 62% of the flux recovery rate for the MoS/PES composite membrane was much higher than the pristine PES membrane (24%). The peroxidase-like properties of MoS were responsible for the enhancement of the superior cleaning performance. The use of HO to trigger the in-situ catalytic function of the MoS nano-enzyme generated more ROS and O for inducing bacterial cells death and facilitating detachment of biofilm. This work will be helpful to provide important insights into developing more effective strategies for biofouling control and cleaning using advanced nanomaterials in membrane-based water treatment processes.

KeywordAntibacterial activity Biofouling Membrane cleaning MoS2 nanosheets
DOI10.1016/j.jece.2023.111571
URLView source
Indexed BySCIE
Language英语English
WOS Research AreaEngineering
WOS SubjectEngineering, Environmental ; Engineering, Chemical
WOS IDWOS:001139405800001
Scopus ID2-s2.0-85178097207
Citation statistics
Document TypeJournal article
Identifierhttp://repository.uic.edu.cn/handle/39GCC9TT/11083
CollectionBeijing Normal-Hong Kong Baptist University
Corresponding AuthorLiu, Yang
Affiliation
1.Joint Research Centre for Protective Infrastructure Technology and Environmental Green Bioprocess,School of Environmental and Municipal Engineering,Tianjin Chengjian University,Tianjin,NO.26, Jinjing Rd, Xiqing District,300384,China
2.Tianjin Key Laboratory of Aquatic Science and Technology,School of Environmental and Municipal Engineering,Tianjin Chengjian University,Tianjin,NO.26, Jinjing Rd, Xiqing District,300384,China
3.Environmental Science Program,Department of Life Sciences,Beijing Normal University-Hong Kong Baptist University United International College,Zhuhai,No. 2000 Jintong Road, Tangjiawan,519087,China
4.Engineering Laboratory of Low-Carbon Unconventional Water Resources Utilization and Water Quality Assurance,College of Environmental Science and Engineering,Nankai University,Tianjin,300350,China
Recommended Citation
GB/T 7714
Huang, Xuanlin,Liu, Yang,Zhao, Yingcanet al. Antibiofouling polyethersulfone ultrafiltration membranes functionalized with MoS2 nanosheets and self-cleaning with hydrogen peroxide[J]. Journal of Environmental Chemical Engineering, 2023, 11(6).
APA Huang, Xuanlin, Liu, Yang, Zhao, Yingcan, Zhang, Xinbo, & Zhang, Xiaoyuan. (2023). Antibiofouling polyethersulfone ultrafiltration membranes functionalized with MoS2 nanosheets and self-cleaning with hydrogen peroxide. Journal of Environmental Chemical Engineering, 11(6).
MLA Huang, Xuanlin,et al."Antibiofouling polyethersulfone ultrafiltration membranes functionalized with MoS2 nanosheets and self-cleaning with hydrogen peroxide". Journal of Environmental Chemical Engineering 11.6(2023).
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